If you want to remove a PC from OneDrive, first make sure all the files
you need are synced to that PC. Do this by opening the OneDrive
System Tray icon. Select Settings > Account > Choose folders.
Check the box to Sync all files and folders in OneDrive, especially
if you unchecked any folders previously.
This action will download any files from OneDrive that don’t already
exist on your PC. This process will take some time, but you can check
the progress by right-clicking the OneDrive System Tray icon to see how
much time is left.
Once all your files are backed up to your PC, right-click the OneDrive
System Tray icon and select Settings. At the Settings tab, uncheck the
box to Start OneDrive automatically when I sign in to Windows.
Then click the Account tab and click the Unlink this PC link. At the
prompt, click the Unlink account button, and now your PC will no
longer sync with OneDrive.
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